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Abstract Charge‐programmed 3D printing enables the fabrication of 3D electronics with lightweight and high precision via selective patterning of metals. This selective metal deposition is catalyzed by Pd nanoparticles that are specifically immobilized onto the charged surface and promises to fabricate a myriad of complex electronic devices with self‐sensing, actuation, and structural elements assembled in a designed 3D layout. However, the achievable property space and the material‐performance correlation of the charge‐programmed printing remain unexplored. Herein, a series of photo‐curable resins are designed for unveiling how the charge and crosslink densities synergistically impact the nanocatalyst‐guided selective deposition in catalytic efficiency and properties of the 3D printed charge‐programmed architectures, leading to high‐quality 3D patterning of solid and liquid metals. The findings offer a wide tunability of the structural properties of the printed electronics, ranging from stiff to extreme flexibility. Capitalizing on these results, the printing and successful application of an ultralight‐weight and deployable 3D multi‐layer antenna system operating at an ultrahigh‐frequency of 19 GHz are demonstrated. 

Architected metamaterials have emerged as a central topic in materials science and mechanics, thanks to the rapid development of additive manufacturing techniques, which have enabled artificial materials with outstanding mechanical properties. This Letter seeks to investigate the elastodynamic behavior of octet truss lattices as an important type of architected metamaterials for high effective strength and vibration shielding. We design, fabricate, and experimentally characterize three types of octet truss structures, including two homogenous structures with either thin or thick struts and one hybrid structure with alternating strut thickness. High elastic wave transmission rate is observed for the lattice with thick struts, while strong vibration mitigation is captured from the homogenous octet truss structure with thin struts as well as the hybrid octet truss lattice, though the underlying mechanisms for attenuation are fundamentally different (viscoelasticity induced dampening vs bandgaps). Compressional tests are also conducted to evaluate the effective stiffness of the three lattices. This study could open an avenue toward multifunctional architected metamaterials for vibration shielding with high mechanical strength. 

Printed low-density materials form microrobots capable of high-speed motion, force output, and self-sensing feedback.